I'd put the figures in and, oops, Calcium turns red (possibly invalid), and "Alkalinity" (as "bicarbonate"). Alkalinity at zero or less is definitely invalid! Looking a bit deeper ... ah, okay, this has entered the "ion mass balancing" bit. It's all grey to discourage users digging this deep (you should see how grey it goes in the area I'm forced to do the "water hardness" codswallop, including "as CaCO3"), oh look, the anions and cations work out the same (0.58mEq/L), so it earned a red splodge ... I think there might have been some human interference there (or a rather surprising coincidence).
Conclusion: That water analysis IS INVALID!
Hi Eric! I'm surprised you've waded into this one. You must have known it was going to have me haul out the behemoth "Water Defuddler"! Okay, its hardly based on space age technology, but hard to argue with all the same. And it really doesn't like "Hardness". Anyway, I do know "chalk" will increase pH. I also know its excrusiatingly difficult to predict what its going to do! You've said "Add some precipitated chalk, stir and take another reading after 5 minutes", which I suppose helps. But this thread is talking of near "real-time" adjustments to pH with "chalk", which is plain fantasy! I wouldn't attempt that with bicarbonate which is far more predictable. Using "chalk" wouldn't even cross my mind.
Cor, haven't had this much fun on "Jim's forum" in ages. Now who might be responsible for the defective water report ... "My water analysis was provided by wallybrew and has subsequently been confirmed independently." ... oops, I'm in trouble now!

"Wally". "Wally", where are you? ... Hang-on, this might take a while ...
[EDIT: Email "wake up" sent ... ]